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• W3044409739 startingPage "2002699" @default.
• W3044409739 abstract "2D materials hold promising potential for novel gas separation. However, a lack of in-plane pores and the randomly stacked interplane channels of these membranes still hinder their separation performance. In this work, ferrocene based-MOFs (Zr-Fc MOF) nanosheets, which contain abundant of in-plane micropores, are synthesized as porous supports to fabricate Zr-Fc MOF supported ionic liquid membrane (Zr-Fc-SILM) for highly efficient CO2 separation. The micropores of Zr-Fc MOF nanosheets not only provide extra paths for CO2 transportation, and thus increase its permeance up to 145.15 GPU, but also endow the Zr-Fc-SILM with high selectivity (216.9) of CO2 /N2 through the nanoconfinement effect, which is almost ten times higher than common porous polymer SILM. Furthermore, based on the photothermal-responsive properties of Zr-Fc MOF, the performance is further enhanced (35%) by light irradiation through a photothermal heating process. This provides a brand new way to design light facilitating gas separation membranes." @default.
• W3044409739 created "2020-07-29" @default.
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• W3044409739 date "2020-07-23" @default.
• W3044409739 modified "2023-10-16" @default.
• W3044409739 title "Photothermal‐Responsive Microporous Nanosheets Confined Ionic Liquid for Efficient CO ₂ Separation" @default.
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• W3044409739 doi "https://doi.org/10.1002/smll.202002699" @default.
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