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- W3044620588 abstract "The methyl-2,2-dicyanoacetate anion is synthesized in an electrospray ionization source through a gas-phase reaction involving tetracyanoethylene and methanol. Photoelectron imaging is used to determine the isomeric form of the product. The photoelectron spectra and angular distributions are consistent with only a single isomer. Additionally, mode-specific vibrational autodetachment is observed. This can be correlated with the emission from a photoexcited dipole-bound state by considering the IR spectrum of the neutral molecule, adding further confirmation of the isomeric form and providing a binding energy of the dipole-bound state. Our experiments show how conventional photoelectron imaging can be used to determine detailed information about gas-phase reaction products." @default.
- W3044620588 created "2020-07-29" @default.
- W3044620588 creator A5058363958 @default.
- W3044620588 creator A5080503123 @default.
- W3044620588 date "2020-07-20" @default.
- W3044620588 modified "2023-09-23" @default.
- W3044620588 title "Gas-Phase Synthesis and Characterization of the Methyl-2,2-dicyanoacetate Anion Using Photoelectron Imaging and Dipole-Bound State Autodetachment" @default.
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- W3044620588 doi "https://doi.org/10.1021/acs.jpclett.0c02036" @default.
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