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- W3044709433 abstract "The high-resistive grain boundaries are the bottleneck for Li+ transport in Li7La3Zr2O12 (LLZO) solid electrolytes. Herein, high-conductive LLZO thin films with cubic phase and amorphous domains between crystalline grains are prepared, via annealing the repetitive LLZO/Li2CO3/Ga2O3 multi-nanolayers at 600 °C for 2 h. The amorphous domains may provide additional vacant sites for Li+, and thus relax the accumulation of Li+ at grain boundaries. The significantly improved ionic conductivity across grain boundaries demonstrates that the high energy barrier for Li+ migration caused by space charge layer is effectively reduced. Benefiting from the Li+ transport paths with low energy barriers, the presented LLZO thin film exhibits a cutting-edge value of ionic conductivity as high as 6.36 × 10-4 S/cm, which is promising for applications in thin film lithium batteries." @default.
- W3044709433 created "2020-07-29" @default.
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- W3044709433 date "2020-07-25" @default.
- W3044709433 modified "2023-10-16" @default.
- W3044709433 title "Reduced Energy Barrier for Li+ Transport Across Grain Boundaries with Amorphous Domains in LLZO Thin Films" @default.
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- W3044709433 doi "https://doi.org/10.1186/s11671-020-03378-x" @default.
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