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- W3044911046 abstract "While the low-index planes of Wurtzite ZnO, such as {0001} and {101¯0} are well-understood, the high-index crystal surfaces have not yet been thoroughly researched despite possessing structural characteristics that make them suitable for many important surface chemistry processes. The high surface energy of high-index ZnO crystal surfaces makes synthesis challenging to achieve due to their instability during crystal growth. In this work, we present a combined experimental and theoretical analysis of growth and photocatalytic activity of ZnO high-index crystal facets. Density functional theory calculations are performed to determine the thermodynamic conditions necessary to stabilize the high-energy semi-polar {112¯2} facets of pyramidal ZnO nanostructures grown via chemical vapor deposition (CVD). The photocatalytic properties of as-synthesized nanopyramidal structures for water splitting applications showed a 73% improved photocatalytic performance compared to CVD-grown hexagonal ZnO nanorods with dominating low-index {101¯0} facets." @default.
- W3044911046 created "2020-07-29" @default.
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- W3044911046 date "2021-01-01" @default.
- W3044911046 modified "2023-10-05" @default.
- W3044911046 title "High-index crystal plane of ZnO nanopyramidal structures: Stabilization, growth, and improved photocatalytic performance" @default.
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- W3044911046 doi "https://doi.org/10.1016/j.apsusc.2020.147326" @default.
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