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• W3045643028 abstract "Abstract The mass transfer in the cathode electrode plays an important role in operating Li-O2 batteries. In this study, a two-dimensional, transient, and isothermal model is developed to investigate the mass transfer in discharging Li-O2 batteries. This model simulates the discharge performance of Li-O2 batteries with various electrolyte concentrations (0.1−1.0M) at various current densities (0.1, 0.3, and 0.5 mA/cm2). The O2 diffusivity and the ionic conductivity and diffusivity of Li+ are altered as the bis(trifluoromethane)sulfonimide lithium salt (LiTFSI) concentration in the electrolyte of tetraethylene glycol dimethyl ether (TEGDME) changes. The distributions of O2, Li+, and lithium peroxide (Li2O2) in the cathode electrode after discharge are calculated using this model. Modeling results show that when the concentration decreases from 0.5 to 0.25M, the discharge capacity of Li-O2 sharply drops at various current densities. The mass transfer of Li+ determines the discharge capacity of Li-O2 batteries with dilute electrolytes (≤0.25 M). In contrast, the O2 supply is dominant regarding the discharge capacity when the electrolyte concentration is larger than 0.5M. The highest discharge capacity (e.g., 6.09 mAh at 0.1 mA/cm2) is achieved using 0.5M electrolyte since it balances mass transfer of O2 and Li+." @default.
• W3045643028 created "2020-08-03" @default.
• W3045643028 creator A5006092337 @default.
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• W3045643028 date "2020-05-11" @default.
• W3045643028 modified "2023-10-14" @default.
• W3045643028 title "A Modeling Study of Discharging Li-O2 Batteries With Various Electrolyte Concentrations" @default.
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• W3045643028 doi "https://doi.org/10.1115/1.4046931" @default.
• W3045643028 hasPublicationYear "2020" @default.
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