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- W3045789122 abstract "Abstract Chiral self‐recognition and self‐discrimination are of vital importance to biological processes. In this work, 2D regular rhombic nanocrystals ( RS ‐NC ) were fabricated through heterochiral self‐discrimination between chiral polynuclear gold(I)‐sulfido complex enantiomers, [( R ‐BINAP) 4 Au 10 S 4 ]Cl 2 ( R ‐Au 10 ) and [( S ‐BINAP) 4 Au 10 S 4 ]Cl 2 ( S ‐Au 10 ), in MeOH without the need for any surfactants or templates. The monitoring of nanocrystals (NCs) formation by TEM and DLS has uncovered the self‐assembly process and shape evolution of the NCs and revealed a screw‐dislocation dictated spiral growth of the rhombic NCs. Upon addition of chiral anions, the morphology of the gold NCs was found to change from rhombic to strip and quasi‐hexagonal nanosheets, arising from reverse and rotational layer‐by‐layer stacking to give the bilayer NCs. By applying a high temperature, rhombic gold nanoisland films were obtained from the rhombic NCs. The current study has provided a simple strategy towards the construction of regular geometric 2D NCs as well as their chiral anion‐tuned and reverse and rotational stacking‐determined morphology change by heterochiral self‐discrimination." @default.
- W3045789122 created "2020-08-03" @default.
- W3045789122 creator A5012250274 @default.
- W3045789122 creator A5043356846 @default.
- W3045789122 creator A5060587180 @default.
- W3045789122 creator A5087631945 @default.
- W3045789122 date "2020-09-15" @default.
- W3045789122 modified "2023-10-18" @default.
- W3045789122 title "Heterochiral Self‐Discrimination‐Driven Supramolecular Self‐Assembly of Decanuclear Gold(I)‐Sulfido Complexes into 2D Nanostructures with Chiral Anions‐Tuned Morphologies" @default.
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- W3045789122 doi "https://doi.org/10.1002/ange.202009728" @default.
- W3045789122 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32725683" @default.
- W3045789122 hasPublicationYear "2020" @default.
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