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• W3046032945 endingPage "350" @default.
• W3046032945 startingPage "341" @default.
• W3046032945 abstract "In this study, rationally designed random copolymers containing highly flexible, low glass transition temperature (Tg) segments are suggested as effective polymeric gelators for high-performance ion gel electrolytes. To this end, a series of poly(styrene-ran-butyl acrylate) copolymers (PS-r-PBAs) is prepared by a one-pot reversible additional-fragmentation chain transfer polymerization. Physically crosslinked ion gel electrolytes are produced by self-assembly when blended with ionic liquids of 1-butyl-3-methylimidazolium bis(trifluoromethyl sulfonyl)imide ([BMI][TFSI]). The properties of gels based on PS-r-PBAs and PS-ran-poly(methyl methacrylate)s (PS-r-PMMAs) are compared at similar molecular conditions. As a result, the effectiveness of the high chain flexibility of butyl acrylate is shown by higher ionic conductivity. The gels with PS-r-PBAs are further optimized in terms of the molecular characteristics of copolymers (e.g., the content of Sty and total molecular weight) and gel composition. The versatility of PS-r-PBA-containing gels as practical electrolyte platforms is demonstrated by preparing all-in-one type electrochromic devices, for which electrochromic ion gels are prepared by incorporating chromophores into the gels. To extend the functionality of the electrochromic devices, dot-shaped electrochromic gel arrays are fabricated for actively controllable smart windows that can reduce the window strike of birds." @default.
• W3046032945 created "2020-08-03" @default.
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• W3046032945 date "2020-10-01" @default.
• W3046032945 modified "2023-09-25" @default.
• W3046032945 title "Impact of chain flexibility of copolymer gelators on performance of ion gel electrolytes for functional electrochemical devices" @default.
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• W3046032945 doi "https://doi.org/10.1016/j.jiec.2020.07.033" @default.
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