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• W3046173792 endingPage "11583" @default.
• W3046173792 startingPage "11577" @default.
• W3046173792 abstract "O2 activation under mild conditions remains a weighty challenge for chemists. Herein we report a study of electrochemical O2 reductive activation catalyzed by FeIII(F20TPP)Cl, by means of cyclic voltammetry and UV–vis spectroelectrochemistry in acidic solutions of N,N-dimethylformamide. Two parallel catalytic pathways have been evidenced occurring at different overpotentials. At high overpotential a classical electron–proton (EPT) pathway where protonation of Fe peroxo ultimately leads to the formation of high-valent Fe oxo species dominates. At low overpotential a proton–electron (PET) pathway involving a hydrosuperoxo species has been identified." @default.
• W3046173792 created "2020-08-03" @default.
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• W3046173792 date "2020-07-29" @default.
• W3046173792 modified "2023-10-18" @default.
• W3046173792 title "Electrocatalytic O₂ Activation by Fe Tetrakis(pentafluorophenyl)porphyrin in Acidic Organic Media. Evidence of High-Valent Fe Oxo Species" @default.
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• W3046173792 doi "https://doi.org/10.1021/acs.inorgchem.0c01379" @default.
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• W3046173792 hasPublicationYear "2020" @default.
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