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- W3046268112 abstract "The first enantioselective total synthesis of (+)-atlanticone C is described. The complex tricyclic protoilludane core was rapidly assembled by a photochemical reaction cascade starting from an easily accessible indanone precursor (3 steps). Optimization of an enantioselective Corey–Bakshi–Shibata reduction permitted a catalytic chiral resolution of the racemic photoproduct (45% over two steps; up to 98% ee). The enantiomerically enriched photoproduct was efficiently transformed into the (+)-enantiomer of atlanticone C (10 steps; 18% yield), and the absolute configuration of naturally occurring (–)-atlanticone C was thereby determined." @default.
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- W3046268112 date "2020-07-31" @default.
- W3046268112 modified "2023-09-27" @default.
- W3046268112 title "Concise Total Synthesis of (+)-Atlanticone C" @default.
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- W3046268112 doi "https://doi.org/10.1055/s-0040-1707215" @default.
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