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- W3046391025 endingPage "126508" @default.
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- W3046391025 abstract "Constructing a lithium metal host is an effective strategy to address the infinite volume change and subsequent vast rupture of solid electrolyte interphase (SEI) for the unsupported Li0/Li+ chemistry, whereas the controllable deposition/dissolution of lithium still need to be improved by the functionalization of the host. Herein, a 3D oxidized polyacrylonitrile fiber network incorporated with LiF (OPAN-LiF) is demonstrated to guide a bottom-up deposition of Li into a flat and dense structure well confined in the host. The oxidation process introduces polar functional groups to the fibers, rendering good wettability with the electrolyte and opulent Li+ access. The incorporation of LiF further tailors lithium deposition and inhibits the formation of dead lithium. The OPAN-LiF electrode can deliver areametric capacity up to 14 mAh cm−2 at 1 mA cm−2 and be stably cycled at current density as high as 5 mA cm−2 with 1 mAh cm−2. Coupled with LiFePO4 cathode, the full cells can present high capacity retention beyond 89% after 1600 cycles at 5C. It is expected that the synthesized 3D functionalized composite scaffolds can be combined with other advanced electrolytes and cathodes to develop high performance lithium metal batteries." @default.
- W3046391025 created "2020-08-07" @default.
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- W3046391025 date "2021-01-01" @default.
- W3046391025 modified "2023-10-14" @default.
- W3046391025 title "Incorporation of LiF into functionalized polymer fiber networks enabling high capacity and high rate cycling of lithium metal composite anodes" @default.
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- W3046391025 doi "https://doi.org/10.1016/j.cej.2020.126508" @default.
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