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• W3046403310 abstract "Pressurized oxy-fuel combustion has been attracting increasing attentions due to its improved efficiency and low cost. The present study reports ignition delay times (IDTs) of pyridine under O2/CO2 atmospheres within a temperature range from 1202 to 1498 K at pressures from 2.2 to 10 bar for equivalence ratios of 0.5, 1.0, and 2.0. The experimental results were compared with the IDTs of pyridine under O2/Ar atmospheres from MacNamara et al.. The comparison results indicate that the IDTs of pyridine under O2/CO2 atmospheres are evident longer than those under O2/Ar atmospheres even at low pressure. A modified kinetic model (HUST pyridine Model) was proposed based on our previous mechanism. HUST pyridine Model predicted well the IDTs under both O2/CO2 and O2/Ar atmospheres obtained in shock tubes and the species profiles under both O2/CO2 and O2/N2 atmospheres obtained in plug flow reactors. HUST pyridine Model, Alzueta Model, and Pyridine LTO Model were evaluated. The results show that the performance of HUST pyridine Model is much better than Alzueta Model, and Pyridine LTO Model. The main reason is that the net reaction rate of C5H5N + O = C5H4N + OH in HUST pyridine Model is much faster than that in Aluzeta Model. The effect of CO2 on the ignition of pyridine at elevated pressures has been analyzed in detail. The oxidation pathways of pyridine are also analyzed at different pressures." @default.
• W3046403310 created "2020-08-07" @default.
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• W3046403310 date "2021-01-01" @default.
• W3046403310 modified "2023-10-11" @default.
• W3046403310 title "A shock tube and modeling study on ignition delay times of pyridine under O2/CO2 atmospheres at elevated pressures" @default.
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• W3046403310 doi "https://doi.org/10.1016/j.proci.2020.06.035" @default.
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