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- W3046688658 abstract "Metals are widely used, from daily life to modern industry. Great efforts have been made to protect the metals with various coatings. However, the well-known conventional electrochemical corrosion induced by cations and the ubiquitous nature of the coffee-ring effect make these processes very difficult. Here, a scheme by two bridges of cations and ethylenediamine (EDA) is proposed to overcome the coffee-ring effect and electrochemical corrosion and experimentally achieve uniform, anticorrosive, and antiabrasive coatings on metallic surfaces. Anticorrosive capability reaches about 26 times higher than that without cation-controlled coatings at 12 h in extremely acidic, high-temperature, and high-humidity conditions and still enhances to 2.7 times over a week. Antiabrasive capability also reaches 2.5 times. Theoretical calculations show that the suspended materials are uniformly adsorbed on the surface mediated by complexed cations through strong cation–metal and cation−π interactions. Notably, the well-known conventional electrochemical corrosion induced by cations is avoided by EDA to control cations solubility in different coating processes. These findings provide a new efficient, cost-effective, facile, and scalable method to fabricate protective coatings on metallic materials and a methodology to study metallic nanostructures in solutions, benefitting practical applications including coatings, printing, dyeing, electrochemical protection, and biosensors." @default.
- W3046688658 created "2020-08-07" @default.
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- W3046688658 date "2020-07-31" @default.
- W3046688658 modified "2023-10-16" @default.
- W3046688658 title "Uniform, Anticorrosive, and Antiabrasive Coatings on Metallic Surfaces for Cation–Metal and Cation−π Interactions" @default.
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- W3046688658 doi "https://doi.org/10.1021/acsami.0c09309" @default.
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