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• W3048129737 abstract "The text-book mechanism of bimolecular nucleophilic aromatic substitutions (SNAr) reactions is a stepwise process that proceeds via a so-called Meisenheimer intermediate. Only recently the alternative, concerted version of this mechanism has gained acceptance as more and more examples thereof have been reported. But so far only isolated examples of concerted SNAr reactions have been described and a coherent picture of when a SNAr reaction proceeds via a stepwise and when via a concerted mechanism has not yet been established. Here key factors are identified that influence the mechanistic choice of SNAr reactions. Moreover, the electron affinity is used as a simple descriptor to make a prediction on whether a given aryl fluoride substrate favors a concerted or stepwise mechanism." @default.
• W3048129737 created "2020-08-13" @default.
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• W3048129737 date "2020-08-07" @default.
• W3048129737 modified "2023-10-02" @default.
• W3048129737 title "Computational Study on the Boundary Between the Concerted and Stepwise Mechanism of Bimolecular S_NAr Reactions" @default.
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• W3048129737 doi "https://doi.org/10.1021/jacs.0c01975" @default.
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