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- W3048223043 endingPage "6570" @default.
- W3048223043 startingPage "6564" @default.
- W3048223043 abstract "Typically, transition metal catalysis enforces the stereodefined outcome of a reaction. Here we disclose the palladium-catalyzed regio- and stereoselective access to allylic ureas/carbamates and their further exploitation to diverse cyclic structures under operationally simple reaction conditions. This protocol features palladium-catalyzed decarboxylative amidation of highly modular VECs with good to excellent yield, minimal waste production, wide substrate scope, and low catalyst loading. In follow-up chemistry, we demonstrated the debenzylation of vinylic imidazolidinones to N-hydroxycyclic ureas and regioselective derivatization towards the facile synthesis of halohydrins and oxiranes under mild reaction conditions in good to excellent yields." @default.
- W3048223043 created "2020-08-13" @default.
- W3048223043 creator A5032532510 @default.
- W3048223043 creator A5042859963 @default.
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- W3048223043 date "2020-01-01" @default.
- W3048223043 modified "2023-09-26" @default.
- W3048223043 title "Palladium-catalyzed regio- and stereoselective access to allyl ureas/carbamates: facile synthesis of imidazolidinones and oxazepinones" @default.
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- W3048223043 doi "https://doi.org/10.1039/d0ob01514h" @default.
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