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• W3048263609 endingPage "110559" @default.
• W3048263609 startingPage "110559" @default.
• W3048263609 abstract "Polarized Raman and optical absorption spectra of oriented Se6 ring clusters incorporated into free spaces of CHA, MOR and AFI zeolite single crystals are studied. The ring orientation was determined via polarization dependence of the bond-bending mode Raman activities which are high in the configuration with both incident and scattered lights polarized parallel to the ring plane. Se6 rings seem to be compressed in CHA cavities, their original D3d symmetry remaining preserved with the ring 3-fold axis orientation along the 3-fold axis of CHA. No symmetry distortion and less compression were found for the Se6 rings in the AFI channels, with their 3-fold axes being oriented along the 3-fold axis of AFI. A noticeable structural distortion is found for Se6 rings in MOR channels which are oriented by their 3-fold axes along the b-axis of MOR. Two broad peaks at 3.1–3.2 eV and 3.5–3.65 eV with rather clear polarization dependence were found in the optical absorption spectra of Se6 rings. Photo-induced Se6 ring fragmentation is demonstrated at illumination with the photon energies of ~1.96 eV and ~2.41 eV at the temperature of ~77 K, formation of Se2− (Se3) and Se8 molecules being observed in CHA and AFI, respectively." @default.
• W3048263609 created "2020-08-13" @default.
• W3048263609 creator A5069173489 @default.
• W3048263609 date "2020-12-01" @default.
• W3048263609 modified "2023-09-23" @default.
• W3048263609 title "Oriented Se6 ring clusters in zeolite single crystals: Polarized Raman microscopy, optical absorption spectra and photo-induced effects" @default.
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• W3048263609 doi "https://doi.org/10.1016/j.micromeso.2020.110559" @default.
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