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- W3048292377 abstract "Greenhouse plant cultivation (GPC) has attracted great attention in recent years, and the search for novel high efficiency far-red emitting phosphor is a crucial task. With this aim in view, in the present paper Ca14Al10Zn6O35:Mn4+ (CAZO:Mn4+) was investigated as a prototype phosphor. By simply incorporating excessive amount of Al, CA10.25ZO:Mn4+ can meet two criteria simultaneously: it has relatively high quantum efficiency (QE) and good thermal stability, which tackle the goal of “killing two birds with one stone”. The internal QE (IQE) could further enhance from 83.9% to 90.0% due to the increased occupancy capability of Mn4+ in [AlO6] octahedron, which is evidenced by solid-state 27Al nuclear magnetic resonance (NMR) and energy dispersive spectra (EDS) measurements. In addition, the Mn4+ concentration-dependent excitation and emission spectra also demonstrate that the optimal doping concentration of Mn4+ in CA10.25ZO host increases from 0.15 to 0.17 mol. Moreover, compared with CA9.85ZO:0.15Mn4+, the thermal stability of CA10.25ZO:0.15Mn4+ improves from 55% to 58% at 150 °C and 38%–45% at 200 °C, respectively. The as-fabricated plant growth LED devices shows better potential to be applied in GPC. This design strategy shown here provides an alternative pathway to further improve the luminescence properties of phosphors." @default.
- W3048292377 created "2020-08-13" @default.
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- W3048292377 date "2020-12-01" @default.
- W3048292377 modified "2023-10-16" @default.
- W3048292377 title "Two targets with one strategy: Insights into the role of aluminum atoms on the luminescence properties and thermal stability in Mn4+-doped calcium aluminozincate phosphor" @default.
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- W3048292377 doi "https://doi.org/10.1016/j.jallcom.2020.156567" @default.
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