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- W3048359767 abstract "The measurement of oxygen potential was conducted at 1673, 1773, and 1873 K for (U 0.623 Pu 0.350 Am 0.027 )O 2 and at 1873 and 1923 K for (U 0.553 Pu 0.285 Am 0.015 Np 0.147 )O 2 by using a thermo-gravimeter and an oxygen sensor. Am inclusion in terms of substituting the U significantly increased the oxygen potential. Similarly, the inclusion of Np as a substitute for U increased the oxygen potential; however, the effect was not as large as that with the Pu addition at the same rate. The results were analyzed via defect chemistry and certain defect formations were suggested in the reducing region and the near-stoichiometric region by plotting the relationship between P O 2 and the deviation from the stoichiometry . The equilibrium constants of the defect reactions were arranged to reproduce the experiment such that Am/Np contents were included in the entropy with coefficients fitting the experimental data." @default.
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- W3048359767 date "2020-12-01" @default.
- W3048359767 modified "2023-09-24" @default.
- W3048359767 title "Oxygen potential measurement of (U,Pu,Am)O2±x and (U,Pu,Am,Np)O2±x" @default.
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- W3048359767 doi "https://doi.org/10.1016/j.jnucmat.2020.152424" @default.
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