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- W3048371319 endingPage "117560" @default.
- W3048371319 startingPage "117560" @default.
- W3048371319 abstract "Abstract Electrochemical activation of persulfate (PS) using Blue-TiO2 nanotubes (Blue-TNT) anode was first attempted for 2,4-dichlorophenoxyacetic acid (2,4-D) decomposition with a low energy consumption of 0.14 kWh m−3, obtaining the rate constant 2.57 and 6.32 times higher than that using boron-doped diamond (BDD) anode and dimensionally stable anode (DSA), respectively. The contribution of responsible radical to 2,4-D degradation on Blue-TNT was 95% from OH while only 2% from SO4 −, differing from that on BDD anode which was ascribed to both OH and non-radical oxidation. The superiority of Blue-TNT anode in PS system was certified by the apparent rate constant which was 6.4, 4.6 and 1.9 times higher than that in the NaNO3, NaClO4 and Na2SO4 electrolyte. Increasing current density and PS concentration and decreasing initial pH accelerated the removal of 2,4-D. The addition of chloride ions (Cl−) enhanced 2,4-D decay, while the presence of bicarbonate (HCO3−) and humic acid (HA) had an inhibition effect on 2,4-D degradation. Overall, electrochemical activation of PS using Blue-TNT was an effective method for contaminants degradation." @default.
- W3048371319 created "2020-08-18" @default.
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- W3048371319 date "2021-01-01" @default.
- W3048371319 modified "2023-10-16" @default.
- W3048371319 title "Enhanced mechanism of 2,4-dichlorophenoxyacetic acid degradation by electrochemical activation of persulfate on Blue-TiO2 nanotubes anode" @default.
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- W3048371319 doi "https://doi.org/10.1016/j.seppur.2020.117560" @default.
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