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- W3048477995 abstract "Efficient electro-reduction of CO2 over metal–organic framework (MOF) materials is hindered by the poor contact between thermally synthesized MOF particles and the electrode surface, which leads to low Faradaic efficiency for a given product and poor electrochemical stability of the catalyst. We report a MOF-based electrode prepared via electro-synthesis of MFM-300(In) on an indium foil, and its activity for the electrochemical reduction of CO2 is assessed. The resultant MFM-300(In)-e/In electrode shows a 1 order of magnitude improvement in conductivity compared with that for MFM-300(In)/carbon-paper electrodes. MFM-300(In)-e/In exhibits a current density of 46.1 mA cm–2 at an applied potential of −2.15 V vs Ag/Ag+ for the electro-reduction of CO2 in organic electrolyte, achieving an exceptional Faradaic efficiency of 99.1% for the formation of formic acid. The facile preparation of the MFM-300(In)-e/In electrode, coupled with its excellent electrochemical stability, provides a new pathway to develop efficient electro-catalysts for CO2 reduction." @default.
- W3048477995 created "2020-08-18" @default.
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- W3048477995 date "2020-09-30" @default.
- W3048477995 modified "2023-10-16" @default.
- W3048477995 title "Quantitative Electro-Reduction of CO<sub>2</sub> to Liquid Fuel over Electro-Synthesized Metal–Organic Frameworks" @default.
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- W3048477995 doi "https://doi.org/10.1021/jacs.0c05913" @default.
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