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- W3048577530 abstract "Chemical looping is a promising combustion technology utilizing the cyclic oxidation and reduction of a metal oxide to transport oxygen for a variety of applications related to carbon capture and storage (CCS). The scalable manufacture of a suitable oxygen carrier is a pivotal aspect of this research field. This work surveys the experimental preparation of CuO and CuO/NiO on SiC and SiO2 substrates for chemical looping with oxygen uncoupling (CLOU) applications. A novel impregnation method that enhances the metal–support interaction to increase dispersion and reduce CuO sintering has been developed in this work. Particles prepared using this method, termed “selective adsorption wet coimpregnation”, exhibited agglomeration resistance and high reactivity over many regeneration cycles. CuO/NiO@SiO2 oxygen carrier (33 wt % CuO, 1 mol of Ni/99 mol of Cu) showed no signs of agglomeration up to 975 °C in fluidized bed testing, cycling between CuO and Cu2O. Thermogravimetric analysis showed no loss in oxygen transport capacity or decrease in kinetics over 100 cycles." @default.
- W3048577530 created "2020-08-18" @default.
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- W3048577530 date "2020-08-11" @default.
- W3048577530 modified "2023-10-18" @default.
- W3048577530 title "Scalable Preparation of Bimetallic Cu/Ni-Based Oxygen Carriers for Chemical Looping" @default.
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- W3048577530 doi "https://doi.org/10.1021/acs.energyfuels.0c01884" @default.
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