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- W3048659967 abstract "Improving electrochemical performance of cathode materials for lithium-ion batteries requires comprehensive understanding of their structural properties which could facilitate or impede the diffusion of lithium during charge-discharge. In order to optimize the structure and improve the electrochemical performance of layered cathode material, the detailed structural evolution as a function of heat treatment temperature in LiNi0.8Co0.1Mn0.1O2 was investigated by in-situ and ex-situ neutron powder diffraction methods. We show that both cycling stability and rate performance of LiNi0.8Co0.1Mn0.1O2 can be improved by performing heat treatment at 400 °C, which is attributed to the optimization of surface structure and the enlargement of c/a ratio. Heat treatment of LiNi0.8Co0.1Mn0.1O2 at higher temperature induces a layered-to-rock-salt structure phase transition accompanied with the precipitation of lithium oxide. A 3D phase diagram, which correlates the high temperature phases and room temperature phases, is constructed. The presentation of comprehensive phase diagrams up to 1000 °C could provide the basis for further research on not only synthesis strategy but also thermal stability in Ni-rich layered cathode materials." @default.
- W3048659967 created "2020-08-18" @default.
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- W3048659967 date "2020-12-01" @default.
- W3048659967 modified "2023-10-14" @default.
- W3048659967 title "Optimizing the structure of layered cathode material for higher electrochemical performance by elucidating structural evolution during heat processing" @default.
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- W3048659967 doi "https://doi.org/10.1016/j.nanoen.2020.105194" @default.
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