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- W3048665172 abstract "Free-electron lasers provide a source of x-ray pulses short enough and intense enough to drive nonlinearities in molecular systems. Impulsive interactions driven by these x-ray pulses provide a way to create and probe valence electron motions with high temporal and spatial resolution. Observing these electronic motions is crucial to understand the role of electronic coherence in chemical processes. A simple nonlinear technique for probing electronic motion, impulsive stimulated x-ray Raman scattering (ISXRS), involves a single impulsive interaction to produce a coherent superposition of electronic states. We demonstrate electronic population transfer via ISXRS using broad bandwidth (5.5 eV full width at half maximum) attosecond x-ray pulses produced by the Linac Coherent Light Source. The impulsive excitation is resonantly enhanced by the oxygen 1s→2π* resonance of nitric oxide (NO), and excited state neutral molecules are probed with a time-delayed UV laser pulse.Received 10 February 2020Revised 21 May 2020Accepted 9 July 2020DOI:https://doi.org/10.1103/PhysRevLett.125.073203© 2020 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasElectronic excitation & ionizationElectronic transitionsSingle- and few-photon ionization & excitationUltrafast phenomenaX-ray beams & opticsNonlinear DynamicsAtomic, Molecular & Optical" @default.
- W3048665172 created "2020-08-18" @default.
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- W3048665172 date "2020-08-11" @default.
- W3048665172 modified "2023-10-16" @default.
- W3048665172 title "Electronic Population Transfer via Impulsive Stimulated X-Ray Raman Scattering with Attosecond Soft-X-Ray Pulses" @default.
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- W3048665172 doi "https://doi.org/10.1103/physrevlett.125.073203" @default.
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