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- W3048749995 abstract "Abstract Herein, the mechanical behaviors of Li 10 GeP 2 S 12 (LGPS) solid electrolytes during electrochemical cycling using operando X‐ray tomography are investigated. It is demonstrated that the bulk mechanical decomposition of LGPS when cycled against lithium is a direct result of electrochemical reduction of the solid electrolyte at the LGPS/Li 0 interface. The reductive decomposition of LGPS during lithium plating results in the formation of low‐density domains at the electrode/electrolyte interface, which impose sufficient mechanical stress on the underlying LGPS to crack the SE pellet. The critical stress developed prior to pellet fracture is significantly lower than the bulk shear modulus of LGPS, suggesting that the electrochemical instability of LGPS dramatically worsens the mechanical stability of the material near the LGPS/Li 0 interface. It is also shown that the application of a highly concentrated liquid electrolyte to the LGPS surface suppresses the reductive decomposition of LGPS, improving both the electrochemical performance and mechanical stability of the bulk LGPS solid electrolyte." @default.
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- W3048749995 date "2020-08-12" @default.
- W3048749995 modified "2023-09-30" @default.
- W3048749995 title "Direct Observation of Interfacial Mechanical Failure in Thiophosphate Solid Electrolytes with Operando X‐Ray Tomography" @default.
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- W3048749995 doi "https://doi.org/10.1002/admi.202000751" @default.
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