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- W3048752728 abstract "Radio-photoluminescence (RPL) materials display a distinct radiation-induced permanent luminescence center, and therefore find application in the detection of ionizing radiation. The current inventory of RPL materials, which were discovered by serendipity, has been limited to a small number of metal-ion-doped inorganic materials. Here we document the RPL of a metal–organic framework (MOF) for the first time: X-ray induced free radicals are accumulated on the organic linker and are subsequently stabilized in the conjugated fragment in the structure, while the metal center acts as the X-ray attenuator. These radicals afford new emission features in both UV-excited and X-ray excited luminescence spectra, making it possible to establish linear relationships between the radiation dose and the normalized intensity of the new emission feature. The MOF-based RPL materials exhibit advantages in terms of the dose detection range, reusability, emission stability, and energy threshold. Based on a comprehensive electronic structure and energy diagram study, the rational design and a substantial expansion of candidate RPL materials can be anticipated." @default.
- W3048752728 created "2020-08-18" @default.
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- W3048752728 date "2020-06-17" @default.
- W3048752728 modified "2023-10-15" @default.
- W3048752728 title "Emergence of a Radical‐Stabilizing Metal–Organic Framework as a Radio‐photoluminescence Dosimeter" @default.
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- W3048752728 doi "https://doi.org/10.1002/anie.202006380" @default.
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