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- W3048778962 abstract "Pyrolytic transition metal nitrogen–carbon (M–N/C) materials are considered as the most promising alternatives for platinum-based catalysts toward oxygen reduction reaction (ORR). As the proton-coupled electron transfer step in ORR has been proven to be a rate-determining step in the M–N/C catalysts, we envisaged that building a protophilic surface might be helpful to enhance the ORR activity. Herein, a polyaniline decoration strategy was put forward and realized to confer the Fe–N/C catalyst with a surface protophilic environment. A 20 mV positive shift in half-wave potential was observed owing to the enriched interfacial proton concentration, corresponding to a tripled turnover frequency under acidic conditions (from 0.46 to 1.28 e·s–1·sites–1). Our work blazed a new path toward the design of M–N/C ORR catalysts, commencing via the ORR kinetics." @default.
- W3048778962 created "2020-08-18" @default.
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- W3048778962 date "2020-08-10" @default.
- W3048778962 modified "2023-10-17" @default.
- W3048778962 title "Construction and Regulation of a Surface Protophilic Environment to Enhance Oxygen Reduction Reaction Electrocatalytic Activity" @default.
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- W3048778962 doi "https://doi.org/10.1021/acsami.0c10155" @default.
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