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- W3048876503 abstract "We present a combined experimental and theoretical study of state-to-state inelastic collisions between NO (X 2Π1/2, j = 1/2, f) radicals and D2 (j = 0, 1, 2, 3) molecules at collision energies of 100 cm-1 and 750 cm-1. Using the combination of Stark deceleration and velocity map imaging, we fully resolve pair-correlated excitations in the scattered molecules. Both spin-orbit conserving and spin-orbit changing transitions in the NO radical are measured, while the coincident rotational excitation (j = 0 → j = 2) and rotational de-excitation (j = 2 → j = 0 and j = 3 → j = 1) in D2 are observed. De-excitation of D2 shows a strong dependence on the spin-orbit excitation of NO. We observe translation-to-rotation energy transfer as well as direct rotation-to-rotation energy transfer at the lowest collision energy probed. The experimental results are in good agreement with cross sections obtained from quantum coupled-channels calculations based on recent NO-D2 potential energy surfaces. The observed trends in the correlated scattering cross sections are understood in terms of the NO-D2 quadrupole-quadrupole interaction." @default.
- W3048876503 created "2020-08-18" @default.
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- W3048876503 date "2020-08-10" @default.
- W3048876503 modified "2023-09-29" @default.
- W3048876503 title "Correlations in rotational energy transfer for NO–D2 inelastic collisions" @default.
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- W3048876503 doi "https://doi.org/10.1063/5.0019472" @default.
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