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- W3048897549 abstract "Cyclic coordination clusters (CCCs) are proving to provide an extra dimension in terms of exotic magnetic behavior as a result of their finite but cyclized chain structures. The Fe18Dy6 CCC is a Single Molecule Magnet with the highest nuclearity among Ln containing clusters. The three isostructural compounds [Fe18Ln6(μ-OH)6(ampd)12(Hampd)12(PhCO2)24](NO3)6·38MeCN for Ln = DyIII (1), LuIII (2), or YIII (3), where H2ampd = 2-amino-2-methyl-1,3-propanediol, are reported. These can be described in terms of the cyclization of six {Fe3Ln(μOH)(ampd)2(Hampd)2(PhCO2)4}+ units with six nitrate counterions to give the neutral cluster. The overall structure consists of two giant Dy3 triangles sandwiching a strongly antiferromagnetically coupled Fe18 ring, leading to a toroidal arrangement of the anisotropy axis of the Dy ions, making this the biggest toroidal arrangement on a molecular level known so far." @default.
- W3048897549 created "2020-08-18" @default.
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- W3048897549 date "2020-08-11" @default.
- W3048897549 modified "2023-09-30" @default.
- W3048897549 title "Inorganic Approach to Stabilizing Nanoscale Toroidicity in a Tetraicosanuclear Fe<sub>18</sub>Dy<sub>6</sub> Single Molecule Magnet" @default.
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- W3048897549 doi "https://doi.org/10.1021/jacs.0c07168" @default.
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