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- W3049242020 endingPage "10810" @default.
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- W3049242020 abstract "This report describes a simple one-pot soft-templating and ammonolysis-free approach to synthesize mesoporous crystalline titanium oxynitride by combining block copolymer-directed self-assembly with metal sol and urea precursors. The Pluronic F127 triblock copolymer was employed to structure-direct titanium-oxo-acetate sol nanoparticles and urea-formaldehyde into ordered hybrid mesostructured monoliths. The hybrid composites were directly converted into mesoporous crystalline titanium oxynitride and retained macroscale monolithic integrity up to 800 °C under nitrogen. Notably, the urea-formaldehyde additive provided nitrogen and rigid support to the inorganic mesostructure during crystallization. The resultant mesoporous titanium oxynitride exhibited good electrochemical catalytic activity toward hydrogen evolution reaction in 1 M KOH aqueous medium under applied bias. Our results suggest an inexpensive and safe pathway to generate ordered mesoporous crystalline metal oxynitride structures suitable for catalyst and energy-storage applications." @default.
- W3049242020 created "2020-08-21" @default.
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- W3049242020 date "2020-08-13" @default.
- W3049242020 modified "2023-09-26" @default.
- W3049242020 title "Mesoporous Titanium Oxynitride Monoliths from Block Copolymer-Directed Self-Assembly of Metal–Urea Additives" @default.
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- W3049242020 doi "https://doi.org/10.1021/acs.langmuir.0c01729" @default.
- W3049242020 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32787003" @default.
- W3049242020 hasPublicationYear "2020" @default.
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