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- W3058876098 abstract "An outstanding metal–organic framework sorbent (Zn-MOF) was prepared using Zn2+ and 3-amino-5-mercapto-1,2,4-triazole to eliminate toxic metal ions from water. Zn-MOF was detected via using Fourier-transform infrared (FTIR) spectroscopy, field-emission scanning electron microscopy (FESEM), Brunauer–Emmett–Teller (BET) analysis, and X-ray photoelectron spectroscopy (XPS). Zn-MOF is stable and has a very large surface area. The uptake properties of Zn-MOF were investigated. The maximum uptake capacity of Zn-MOF for Pb, Hg, and As ions was 1097, 32, and 718 mg/g, respectively. This was obtained at pH = 4, 5, and 6, respectively. The adsorption data is in good agreement with the Langmuir and pseudo-second-order rate models, indicating that the uptake process of Zn-MOF for toxic metal ions was a single layer uptake on a uniform surface via exchange of valence electrons. Thermodynamics shows that the uptake process is autogenic and endothermic. Zn-MOF can be reused at least 6 times. Mercury and lead strongly coordinated with Zn-MOF. The interaction between arsenic and Zn-MOF is weak chemical coordination and ion exchange. Zn-MOF has wide application prospects for toxic metal ion elimination." @default.
- W3058876098 created "2020-08-24" @default.
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- W3058876098 date "2020-08-19" @default.
- W3058876098 modified "2023-10-14" @default.
- W3058876098 title "Preparation of a Novel Zn(II)-Imidazole Framework as an Efficient and Regenerative Adsorbent for Pb, Hg, and As Ion Removal From Water" @default.
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- W3058876098 doi "https://doi.org/10.1021/acsami.0c10298" @default.
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