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- W3066221093 abstract "Significance Colloidal nanocrystals with defined sizes and shapes are ideal building blocks for nanofabrication. However, the ability to arbitrarily arrange them on surfaces with control over their orientation remains elusive. Here we report a shallow-template-assisted DNA-mediated assembly strategy to precisely arrange colloidal nanocrystals on surfaces, with single-particle control across submillimeter areas. In addition, the oligonucleotide bonds between the nanocrystals and substrate can be reversibly expanded and contracted enabling postsynthetic tunability of the assembled structures. Using this approach, we synthesized a nanocrystal-based, dynamically tunable metasurface (an anomalous reflector), thereby illustrating the potential for unique device construction via DNA programmable assembly." @default.
- W3066221093 created "2020-08-24" @default.
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- W3066221093 date "2020-08-17" @default.
- W3066221093 modified "2023-10-02" @default.
- W3066221093 title "Device-quality, reconfigurable metamaterials from shape-directed nanocrystal assembly" @default.
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- W3066221093 doi "https://doi.org/10.1073/pnas.2006797117" @default.
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