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• W3080128087 abstract "Synthesis of catalysts with high activity for hydrogen evolution reaction (HER) has been a hot topic in electrocatalysis. In this paper, using MIL-88A(Fe) metal-organic complex, polyoxometalate (POM) and H2PtCl6 as starting materials, hierarchic and low Pt0-loading micro-rods (denoted as Pt-POMFe, i.e. Pt-PW12Fe or Pt-PMo12Fe) have been synthesized, in which the Pt0 nanoparticles can be stabilized by POM. The Pt-PW12Fe micro-rod containing [PW12O40]3- polyoxoanion component (0.30% Pt0-loading) which retains the spindle structure of its parent MIL-88A(Fe) exhibits a low overpotential of 28 mV at current density of 10 mA·cm−2 for HER that is close to the electrocatalytic effect of commercial Pt/C (ca. 20% Pt0-loading). Such high electrocatalytic reactivity is mainly caused by the synergistic effect of the three components of POM, Pt0, and Fe3O4@C. The structure effectively increases the active sites of the catalyst and improves its conductivity and stability. The Pt-POMFe catalyst extends a new family of MOF-POM functional materials and provides a new concept to the design and synthesis of highly-efficient and low-cost electrocatalyst for hydrogen production." @default.
• W3080128087 created "2020-09-01" @default.
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• W3080128087 date "2020-08-26" @default.
• W3080128087 modified "2023-10-14" @default.
• W3080128087 title "Ultralow Pt⁰ loading on MIL-88A(Fe) derived polyoxometalate-Fe₃O₄@C micro-rods with highly-efficient electrocatalytic hydrogen evolution" @default.
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• W3080128087 doi "https://doi.org/10.1080/00958972.2020.1809656" @default.
• W3080128087 hasPublicationYear "2020" @default.
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