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• W3080212912 abstract "We show that a polar, pseudo-Jahn-Teller instability exists for the underbonded rare-earth $A$-site cations in the quadruple perovskite ${mathrm{Dy}}_{1ensuremath{-}ensuremath{delta}}{mathrm{Mn}}_{7+ensuremath{delta}}{mathrm{O}}_{12}$, which leads to the spontaneous formation of a dipolar glass. This observation alone expands the applicability of pseudo-Jahn-Teller physics in perovskite-derived materials, for which it is typically confined to $B$-site cations. We demonstrate that the dipolar glass order parameter is coupled to a ferrimagnetic order parameter via strain, leading to a first order magnetostructural phase transition that can be tuned by magnetic field. This phenomenology may emerge in a broad range of perovskite-derived materials in which $A$-site cation ordering and octahedral tilting are mutually tied to meet the criteria of structural stability." @default.
• W3080212912 created "2020-09-01" @default.
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• W3080212912 date "2020-08-26" @default.
• W3080212912 modified "2023-09-26" @default.
• W3080212912 title "Emergence of a Magnetostructural Dipolar Glass in the Quadruple Perovskite <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi>Dy</mml:mi></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mo>−</mml:mo><mml:mi>δ</mml:mi></mml:mrow></mml:msub><mml:mrow><mml:msub><mml:mrow><mml:mi>Mn</mml:mi></mml:mrow><mml:mrow><mml:mn>7</mml:mn><mml:mo>+</mml:mo><mml:mi>δ</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>…" @default.
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• W3080212912 doi "https://doi.org/10.1103/physrevlett.125.097601" @default.
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