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• W3080456444 abstract "We investigate the pulse length dependence of the third-order nonlinear response of a gold film using pulse widths between 325 and 650 fs at λ=1320 nm via a sensitive cut-pulse technique that measures background-free self-phase modulation. We find a cubic dependence of the transmitted nonlinear power on incident peak intensity that is independent of the pulse width in this range to within experimental accuracy. We estimate a value of χ3=8±3×10−18 m2/V2 by fitting experimental data to numerical simulations accounting for both losses and reflections at each film interface. These results provide valuable insights into near-infrared nonlinear plasmonic device designs." @default.
• W3080456444 created "2020-09-01" @default.
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• W3080456444 date "2020-08-17" @default.
• W3080456444 modified "2023-10-14" @default.
• W3080456444 title "Pulse length dependent near-infrared ultrafast nonlinearity of gold by self-phase modulation" @default.
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• W3080456444 doi "https://doi.org/10.1063/5.0020588" @default.
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