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- W3080495535 abstract "Al atoms generally adopt the +3 oxidation state and form stoichiometric oxides such as Al2O3 in the bulk phase. Among small cationic gas-phase clusters, near-stoichiometric clusters such as Al3O4+, Al3O5+, Al4O6+, Al4O7+, Al5O7+, and Al5O8+ have been readily generated in experimental studies. However, when a single Au atom was included in the clusters, oxygen-deficient clusters such as AuAl4O5+ were formed in high abundance; in these clusters, the Au atom accepted electron density from the Al atoms. The geometrical structures and atomic charges in the clusters suggest that a single Au atom can substitute for O atoms in Al oxide clusters. This propensity originates from the high electron and low oxygen affinities, which, together, constitute an unusual property of Au." @default.
- W3080495535 created "2020-09-01" @default.
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- W3080495535 date "2020-08-23" @default.
- W3080495535 modified "2023-10-04" @default.
- W3080495535 title "Substitution of O with a Single Au Atom as an Electron Acceptor in Al Oxide Clusters" @default.
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- W3080495535 doi "https://doi.org/10.1021/acs.jpca.0c06269" @default.
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