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• W3080525097 abstract "We performed angle-resolved photoemission spectroscopy (ARPES) of bulk 2H-WSe2 for different crystal orientations linked to each other by time-reversal symmetry. We introduce a new observable called time-reversal dichroism in photoelectron angular distributions (TRDAD), which quantifies the modulation of the photoemission intensity upon effective time-reversal operation. We demonstrate that the hidden orbital pseudospin texture leaves its imprint on TRDAD, due to multiple orbital interference effects in photoemission. Our experimental results are in quantitative agreement with both the tight-binding model and state-of-the-art fully relativistic calculations performed using the one-step model of photoemission. While spin-resolved ARPES probes the spin component of entangled spin-orbital texture in multiorbital systems, we unambiguously demonstrate that TRDAD reveals its orbital pseudospin texture counterpart.Received 2 June 2020Accepted 13 October 2020Corrected 14 December 2020DOI:https://doi.org/10.1103/PhysRevLett.125.216404Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI. Open access publication funded by the Max Planck Society.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCrystal symmetryElectronic structureFirst-principles calculationsPhysical SystemsTransition metal dichalcogenidesTechniquesAngle-resolved photoemission spectroscopyKorringa-Kohn-Rostoker methodPhotoemission spectroscopyCondensed Matter, Materials & Applied Physics" @default.
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• W3080525097 date "2020-11-20" @default.
• W3080525097 modified "2023-10-16" @default.
• W3080525097 title "Revealing Hidden Orbital Pseudospin Texture with Time-Reversal Dichroism in Photoelectron Angular Distributions" @default.
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• W3080525097 doi "https://doi.org/10.1103/physrevlett.125.216404" @default.
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