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- W30805722 abstract "FT-IR spectroscopy has been used to study the surface species formed during the interaction of CO with Ru and Ir supported on highly dealuminated zeolite (US-Ex). With both oxidized and reduced Ru/US-Ex a well defined Ru tricarbonyl could be identified with bands at 2152, 2091 and 2086 cm−1 indicating a slightly distorted C3V structure. Evacuation at 473 K results in the formation of a Ru dicarbonyl with bands at 2092 and 2031 cm−1. Ir(CO)2/US-Ex with bands at 2108 and 2037 cm−1 was obtained after an interaction of CO with oxidized Ir/US-Ex. Different to Rh and Ru, reduced Ir did not form a well defined surface carbonyl on US-Ex. TPR-TPO was used to explain these differences and the increasing temperature (Rh<Ru<Ir) of CO interaction, which is necessary to form the well defined carbonyls on the oxidized samples." @default.
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- W30805722 date "1991-01-01" @default.
- W30805722 modified "2023-09-25" @default.
- W30805722 title "The Formation of Well Defined Surface Carbonyls of RU and IR with Highly Dealuminated Zeolite Y as Matrix" @default.
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- W30805722 doi "https://doi.org/10.1016/s0167-2991(08)61572-4" @default.
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