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• W3080996856 endingPage "119475" @default.
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• W3080996856 abstract "Although two-dimensional graphitic carbon nitride (2D g-C3N4) and corresponding heterostructures have been widely synthesized for photocatalysis, it is still challenging to obtain 2D g-C3N4 at large-scale and also achieve high quantum efficiency. Here we report a subtractive manufacturing method mediated by Nb2O5 to mass-produce high quality Nb2O5/2D g-C3N4 and pure 2D g-C3N4. Nb2O5/2D g-C3N4 and 2D g-C3N4 both show efficient photocatalytic hydrogen evolution performance, in which the optimal Nb2O5/2D g-C3N4 exhibits high external quantum efficiency (50.65 % and 14.75 % at 405 nm and 420 nm). The origin of the high efficiency can be ascribed to two aspects: (i) nanostructure engineering forming 2D structure can shorten the charge migration distance; (ii) Nb2O5/2D g-C3N4 with strong electric coupling can further accelerate the charge transfer driven by the built-in electric field formed in Type II heterostructure. This work presents a case study to realize high-yield synthesis and high catalytic performance simultaneously over g-C3N4." @default.
• W3080996856 created "2020-09-01" @default.
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• W3080996856 date "2021-02-01" @default.
• W3080996856 modified "2023-10-16" @default.
• W3080996856 title "Large-scale production of ultrathin carbon nitride-based photocatalysts for high-yield hydrogen evolution" @default.
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• W3080996856 doi "https://doi.org/10.1016/j.apcatb.2020.119475" @default.
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