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- W3082142854 abstract "Explaining the dynamics of gas-saturated live petroleum in deep water remains a challenge. Recently, Pesch et al. [ Environ. Eng. Sci. 2018, 35 (4), 289-299] reported laboratory experiments on methane-saturated oil droplets under emulated deep-water conditions, providing an opportunity to elucidate the underlying dynamical processes. We explain these observations with the Texas AM aqueous dissolution; and densities and volumes of liquid oil droplets, gas bubbles, and two-phase droplet-bubble pairs. TAMOC reveals that aqueous dissolution removed >95% of the methane from ∼3.5 mm live oil droplets within 14.5 min, prior to gas bubble formation, during the experiments of Pesch et al. Additional simulations indicate that aqueous dissolution, fluid density changes, and gas-oil phase transitions (ebullition, condensation) may all contribute to the fates of live oil and gas in deep water, depending on the release conditions. Illustrative model scenarios suggest that 5 mm diameter gas bubbles released at a <470 m water depth can transport methane, ethane, and propane to the water surface. Ethane and propane can reach the water surface from much deeper releases of 5 mm diameter live oil droplets, during which ebullition occurs at water depths of <70 m." @default.
- W3082142854 created "2020-09-08" @default.
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- W3082142854 date "2020-08-28" @default.
- W3082142854 modified "2023-10-05" @default.
- W3082142854 title "Dynamics of Live Oil Droplets and Natural Gas Bubbles in Deep Water" @default.
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- W3082142854 doi "https://doi.org/10.1021/acs.est.9b06242" @default.
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