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• W3082146523 endingPage "22469" @default.
• W3082146523 startingPage "22465" @default.
• W3082146523 abstract "Main-group element indium (In) is a promising electrocatalyst which triggers CO2 reduction to formate, while the high overpotential and low Faradaic efficiency (FE) hinder its practical application. Herein, we rationally design a new In single-atom catalyst containing exclusive isolated Inδ+ -N4 atomic interface sites for CO2 electroreduction to formate with high efficiency. This catalyst exhibits an extremely large turnover frequency (TOF) up to 12500 h-1 at -0.95 V versus the reversible hydrogen electrode (RHE), with a FE for formate of 96 % and current density of 8.87 mA cm-2 at low potential of -0.65 V versus RHE. Our findings present a feasible strategy for the accurate regulation of main-group indium catalysts for CO2 reduction at atomic scale." @default.
• W3082146523 created "2020-09-08" @default.
• W3082146523 creator A5014698348 @default.
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• W3082146523 creator A5076411026 @default.
• W3082146523 creator A5079594267 @default.
• W3082146523 creator A5085142676 @default.
• W3082146523 date "2020-10-06" @default.
• W3082146523 modified "2023-10-17" @default.
• W3082146523 title "Design of a Single‐Atom Indium ^δ+ –N ₄ Interface for Efficient Electroreduction of CO ₂ to Formate" @default.
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