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• W3083522195 abstract "The synthesis, structure, and physical properties of Y 5 Ru 2 O 12 , a new member of the Ln 5 B 2 O 12 class (Ln = lanthanide, B = Ru, Re, Mo) are reported. Single crystals of Y 5 Ru 2 O 12 are synthesized using a high‐temperature, high‐pressure (700 °C, 200 MPa) hydrothermal method. The structure features edge‐sharing RuORu 1D chains of distorted RuO 6 octahedra. The YO n ( n = 6 and 7) polyhedral groups bridge RuORu chains across the unit cell by forming a complex 3D structure. The RuORu chains contain alternating shorter and longer RuRu distances along the chain. Single crystal neutron diffraction shows streak‐like diffuse scattering along the H ‐direction, due to stacking faults. Temperature‐dependent anisotropic magnetic measurements reveal a broad feature over a wide temperature range, with a maximum at ≈70 K indicating potential short‐range ordering, with canted antiferromagnetic behavior below 30 K. The dominant magnetic interactions are antiferromagnetic with a large negative Weiss temperature θ ≈ −200 K. The compound has an effective magnetic moment that is anomalously large for this class of compounds (≈4 μ B Ru −1 ), and a phenomenological spin Hamiltonian describing the unusual anisotropic magnetization of Y 5 Ru 2 O 12 is proposed." @default.
• W3083522195 created "2020-09-11" @default.
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• W3083522195 date "2020-09-21" @default.
• W3083522195 modified "2023-09-23" @default.
• W3083522195 title "Stacking Faults and Short‐Range Magnetic Correlations in Single Crystal Y₅Ru₂O₁₂: A Structure with Ru^+4.5 One‐Dimensional Chains" @default.
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• W3083522195 doi "https://doi.org/10.1002/pssb.202000197" @default.
• W3083522195 hasPublicationYear "2020" @default.
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