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• W3083893722 startingPage "43805" @default.
• W3083893722 abstract "The rational design and optimization of solid polymer electrolytes (SPEs) are critical for the application of safety and high efficiency lithium ion batteries (LIBs). Herein, we synthesized a novel poly(ethylene oxide) (PEO)-based SPE (PEO@AF SPE) with a cross-linking network by the introduction of alginate fiber (AF) membranes. Depending on the high-strength supporting AF skeleton and the cross-linking network formed by hydrogen bonds between the PEO matrix and AF skeleton, the obtained PEO@AF SPE exhibits an excellent tensile strength of 3.71 MPa, favorable heat resistance (close to 120 °C), and wide electrochemical stability window (5.2 V vs Li/Li+). Meanwhile, the abundant oxygen-containing groups in alginate macromolecular and the three-dimensional (3D) porous structure of the AF membrane can greatly increase Li+ anchor points and provide more Li+ migration pathways, leading to the enhancement of Li+ conduction and interfacial stability between the SPE and Li anode. Furthermore, the assembled LiFePO4/PEO@AF SPE/Li cells also exhibit satisfactory electrochemical performance. These results reveal that PEO incorporating with AFs can boost the mechanical strength, thermostability, and electrochemical properties of the SPE simultaneously. Furthermore, one will expect that the newly designed PEO@AF SPE with cross-linked networks thus provides the possibility for future applications of safety and high-performance LIBs." @default.
• W3083893722 created "2020-09-14" @default.
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• W3083893722 date "2020-09-08" @default.
• W3083893722 modified "2023-10-02" @default.
• W3083893722 title "Three-Dimensional Porous Alginate Fiber Membrane Reinforced PEO-Based Solid Polymer Electrolyte for Safe and High-Performance Lithium Ion Batteries" @default.
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• W3083893722 doi "https://doi.org/10.1021/acsami.0c13039" @default.
• W3083893722 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32897049" @default.
• W3083893722 hasPublicationYear "2020" @default.
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