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• W3084054041 abstract "利用间歇性可再生能源电转化二氧化碳和一氧化碳制备多 碳工业原料和燃料能够完善碳循环. 然而, 二氧化碳转化为乙酸的 法拉第效率难以满足大规模应用的要求. 研究发现, 调控铜的局域 电子结构至正价态, 以及使用一氧化碳作为反应气均能够提高多 碳产物的选择性. 因此, 我们提出杂原子调控策略, 用于调节催化 剂表面活性位点的氧化态. 密度泛函理论研究表明, 掺杂氮原子调 控正价态铜位点, 在热力学上有利于形成中间体*CCO, 进而生成 乙酸. 我们进一步利用溶剂热法合成氮掺杂的铜催化剂, 并通过软 X射线吸收谱和X射线光电子能谱证实催化剂表面存在大量正价态 铜位点. 同时, 该催化剂在一氧化碳还原反应中实现了42%的乙酸 法拉第效率和已知最高的乙酸偏电流密度180 mA cm−2." @default.
• W3084054041 created "2020-09-14" @default.
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• W3084054041 date "2020-09-07" @default.
• W3084054041 modified "2023-10-09" @default.
• W3084054041 title "N-modulated Cu+ for efficient electrochemical carbon monoxide reduction to acetate" @default.
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• W3084054041 doi "https://doi.org/10.1007/s40843-020-1440-6" @default.
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