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- W3084256106 abstract "Abstract Sulfur-containing functional π-conjugated cores play key roles in materials science, mostly due to their unique electrochemical and photophysical properties. Among these, the excellent electron donor tetrathiafulvalene (TTF) has occupied a central position since the emergence of organic electronics. Peripheral C–H modification of this highly useful sulfur-containing motif has resulted in the efficient creation of new molecules that expand the applications of TTFs. This Short Review begins with the development of the palladium-catalyzed direct C–H arylation of TTF. Subsequently, it summarizes the applications of this efficient C–H transformation for the straightforward synthesis of useful TTF derivatives that are employed in a variety of research fields, demonstrating that the development of a new reaction can have a significant impact on chemical science. 1 Introduction 2 Development of the Palladium-Catalyzed Direct C–H Arylation of TTF 3 Synthesis of TTF-Based Tetrabenzoic Acid and Tetrapyridine for MOFs 4 Synthesis of TTF-Based Tetrabenzaldehyde and Tetraaniline for COFs 5 Tetraarylation of TTFAQ 6 Synthesis of Multistage-Redox TTF Derivatives 7 Miscellaneous Examples 8 Conclusions" @default.
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- W3084256106 date "2020-09-08" @default.
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- W3084256106 title "Catalytic C–H Arylation of Tetrathiafulvalenes for the Synthesis of Functional Materials" @default.
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