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• W3085206884 abstract "The cobalt-based phosphates are important and efficient catalysts for improving the activity of oxygen evolution reaction (OER), which is an essential reaction in water splitting. Here, a series of S-doped cobalt-based phosphate nanomaterials are synthesized through a simple co-precipitation process. It is found that the amorphous S-doped cobalt-iron phosphate (S-doped Co-Fe-Pi) nanosheets with an Co/Fe ratio of 6.9:1 can display the best electrochemical activity for OER, requiring an overpotential of only 273 mV to drive the current density of 10 mA cm−2 in 1M KOH. As a highly efficient catalyst, both the structure features and the electrocatalytic performance of S-doped Co-Fe-Pi catalysts are discussed in this work. More importantly, the OER performance of the catalysts affected by thiophosphate anions and Fe incorporated cations is investigated. Finally, it is suggested that the outstanding activity can be attributed to not only the porous nanostructure existing in amorphous morphology, but also the proper electronic state of Co atoms induced by the decoration of Fe and S atoms." @default.
• W3085206884 created "2020-09-21" @default.
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• W3085206884 date "2020-12-01" @default.
• W3085206884 modified "2023-10-16" @default.
• W3085206884 title "S-doped Co-Fe-Pi nanosheets as highly efficient oxygen evolution electrocatalysts in alkaline media" @default.
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• W3085206884 doi "https://doi.org/10.1016/j.electacta.2020.137123" @default.
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