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- W3085720080 abstract "We demonstrate three-dimensional (3D) field-free alignment of the prototypical non-rotation-symmetric molecule indole using elliptically polarized, shaped, off-resonant laser pulses. A truncated laser pulse is produced using a combination of extreme linear chirping and controlled phase and amplitude shaping using a spatial-light-modulator (SLM) based pulse shaper of a broadband laser pulse. The angular confinement is detected through velocity-map imaging of H$^+$ and C$^{2+}$ fragments resulting from strong-field ionization and Coulomb explosion of the aligned molecules by intense femtosecond laser pulses. The achieved three-dimensional alignment is characterized by comparing the result of ion-velocity-map measurements for different alignment directions and for different times during and after the alignment laser pulse to accurate computational results. The achieved strong three-dimensional field-free alignment of $langlecos^{2}deltarangle=0.89$ demonstrates the feasibility of both, strong three-dimensional alignment of generic complex molecules and its quantitative characterization." @default.
- W3085720080 created "2020-09-21" @default.
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- W3085720080 date "2020-09-17" @default.
- W3085720080 modified "2023-09-27" @default.
- W3085720080 title "Picosecond pulse-shaping for strong three-dimensional field-free alignment of generic asymmetric-top molecules" @default.
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