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• W3087079380 abstract "Owing to the diminishing resources and growing awareness of environmental issues, significant scientific attention has been paid to the development of physical gel materials using renewable and low-cost natural resources. Inspired by the strengthened mechanism of double-network and nanocomposite (NC) gels, we report a facile and green method to realize a mechanically stiff, fatigue-resistant, and adhesive-debranched waxy corn starch/poly(vinyl alcohol) double-crosslinked NC gel (W-Gel) skeleton material with dynamic noncovalent bonds. The in situ formation of debranched starch nanoparticles leads to self-assembly into three-dimensional waxberry-like microspheres, which act as physical cross-linkers by embedding themselves within network skeleton structures. The resulting hydrogel exhibited an excellent mechanical behavior, including a good stretchability over 1200% strain, a maximum compressive strength of up to 780.7 ± 27.8 kPa, and the ability to sustain as much weight as 4.6 kg (about 2000 times its own weight). Notably, the recovery efficiency exceeded 93% after the 60th compressive successive loading-unloading cycle at 50% strain. The hydrogel successfully adhered onto soft and hard substrates, such as skins, plastics, gauzes, glasses, and metals, manifesting in long-term, stable, sustained release of epigallocatechin gallate (EGCG). The EGCG-loaded W-Gels exhibited predominant antibacterial activity against both Gram-positive bacteria (Staphylococcus aureus) and Gram-negative bacteria (Escherichia coli and Salmonella typhus)." @default.
• W3087079380 created "2020-09-25" @default.
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• W3087079380 date "2020-09-21" @default.
• W3087079380 modified "2023-10-03" @default.
• W3087079380 title "In Situ Self-Assembly of Nanoparticles into Waxberry-Like Starch Microspheres Enhanced the Mechanical Strength, Fatigue Resistance, and Adhesiveness of Hydrogels" @default.
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• W3087079380 doi "https://doi.org/10.1021/acsami.0c10327" @default.
• W3087079380 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/32955240" @default.
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