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- W3087143580 endingPage "119563" @default.
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- W3087143580 abstract "Abstract Herein, two-dimension (2D) δ-MnO2-modified porous g-C3N4/micro-mesoporous titanium phosphate (MO-CN/TiP) nanocomposites have been controllably fabricated by a two-step solvothermal process. The amount-optimized MO-CN/TiP nanocomposite exhibits greatly improved photocatalytic CO oxidation performance (87%) compared with corresponding bare TiP and CN/TiP, even superior to the commercial P25 TiO2. Based on the experimental results of time-resolved surface photovoltage responses, photocurrent action spectra, and electron paramagnetic resonance signals, it is clearly confirmed that the exceptional photoactivity is mainly attributed to the great promotion in the Z-scheme charge transfer in resultant dimension-matched CN/TiP nanocomposite and in the O2 activation via the modified MO. The porous structure favorable to increase the specific surface areas and to facilitate the mass diffusion and the extended visible-light absorption also contribute to the photoactivity enhancement. Moreover, it is uncovered by the in-situ diffuse reflectance fourier transform infrared spectra that CO is previously adsorbed by the formed OH OC intermediate with the surface hydroxyls and then oxidized." @default.
- W3087143580 created "2020-09-25" @default.
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- W3087143580 date "2021-03-01" @default.
- W3087143580 modified "2023-09-24" @default.
- W3087143580 title "Porous two-dimension MnO2-C3N4/titanium phosphate nanocomposites as efficient photocatalsyts for CO oxidation and mechanisms" @default.
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- W3087143580 doi "https://doi.org/10.1016/j.apcatb.2020.119563" @default.
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