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- W3087196714 endingPage "2007172" @default.
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- W3087196714 abstract "Poly(ethylene oxide) (PEO)-based electrolytes are promising for all-solid-state batteries but can only be used above room temperature due to the high-degree crystallization of PEO and the intimate affinity between ethylene oxide (EO) chains and lithium ions. Here, a homogeneous-inspired design of PEO-based solid-state electrolytes with fast ion conduction is proposed. The homogeneous PEO-based solid-state electrolyte with an adjusted succinonitrile (SN) and PEO molar ratio simultaneously suppresses the PEO crystallization and mitigates the affinity between EO and Li+. By adjusting the molar ratio of SN to PEO (SN:EO ≈ 1:4), channels providing fast Li+ transport are formed within the homogeneous solid-state polymer electrolyte, which increases the ionic conductivity by 100 times and enables their application at a low temperature (0–25 °C), together with the uniform lithium deposition. This modified PEO-based electrolyte also enables a LiFePO4 cathode to achieve a superior Coulombic efficiency (>99%) and have a long life (>750 cycles) at room temperature. Moreover, even at a low temperature of 0 °C, 82% of its room-temperature capacity remains, demonstrating the great potential of this electrolyte for practical solid-state lithium battery applications." @default.
- W3087196714 created "2020-09-25" @default.
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- W3087196714 date "2020-09-16" @default.
- W3087196714 modified "2023-10-16" @default.
- W3087196714 title "Homogeneous and Fast Ion Conduction of PEO‐Based Solid‐State Electrolyte at Low Temperature" @default.
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- W3087196714 doi "https://doi.org/10.1002/adfm.202007172" @default.
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