Matches in SemOpenAlex for { <https://semopenalex.org/work/W3087218857> ?p ?o ?g. }
- W3087218857 endingPage "118735" @default.
- W3087218857 startingPage "118735" @default.
- W3087218857 abstract "Protons transport profoundly affects diverse fields from proton-exchange membrane fuel cells to storing liquid hydrogen. Recent advances have extended proton-exclusive transport to the two-dimensional channels that use hydrous mechanisms for fast proton transport, where the main challenge is the limited selectivity. However, the physical and chemical properties of 2D nanosheets like GO have the potential to implement full selective and ultrafast proton transport. Here, we uncover the physical potential of anhydrous proton transfer mechanism inside two-dimensional space between graphene nanosheets to exploit the exceptional full proton-selective ability and ultrafast conveyance speed of the Grotthuss mechanism. Reactive molecular dynamics simulations illustrate that the interlayer space between two graphene oxide nanosheets, carpeted with hydroxyl functional groups as additional hopping stages to enable the Grotthuss mechanism, can convey protons without water. Further, we dissect three essential factors that provide a deeper insight into ultrafast proton transport: (i) transitional phase to full anhydrous transport, (ii) outlet size for containing undesired species, and (iii) elastic behavior of the membranes under external strain. Our results show that changes in surface geometry can dramatically increase the diffusion rate in the presence of a small electric field by ~70% compared to hydrous transport. These findings can be used not only to guide the efforts in manufacturing a new generation of sustainable nanochannels but also to advance the pioneering technologies revolving around hydrogen." @default.
- W3087218857 created "2020-09-25" @default.
- W3087218857 creator A5007737530 @default.
- W3087218857 creator A5008884053 @default.
- W3087218857 creator A5027923393 @default.
- W3087218857 creator A5043481897 @default.
- W3087218857 creator A5046889467 @default.
- W3087218857 creator A5061541506 @default.
- W3087218857 date "2021-01-01" @default.
- W3087218857 modified "2023-10-11" @default.
- W3087218857 title "Insight from perfectly selective and ultrafast proton transport through anhydrous asymmetrical graphene oxide membranes under Grotthuss mechanism" @default.
- W3087218857 cites W1569308213 @default.
- W3087218857 cites W1859169177 @default.
- W3087218857 cites W1907589562 @default.
- W3087218857 cites W1965460216 @default.
- W3087218857 cites W1974371866 @default.
- W3087218857 cites W2002295407 @default.
- W3087218857 cites W2010922597 @default.
- W3087218857 cites W2019465613 @default.
- W3087218857 cites W2022336433 @default.
- W3087218857 cites W2026291014 @default.
- W3087218857 cites W2036260386 @default.
- W3087218857 cites W2037684576 @default.
- W3087218857 cites W2048726254 @default.
- W3087218857 cites W2055638681 @default.
- W3087218857 cites W2108098890 @default.
- W3087218857 cites W2110061367 @default.
- W3087218857 cites W2117100297 @default.
- W3087218857 cites W2118849046 @default.
- W3087218857 cites W2155155530 @default.
- W3087218857 cites W2156200742 @default.
- W3087218857 cites W2156357247 @default.
- W3087218857 cites W2163822354 @default.
- W3087218857 cites W2318370903 @default.
- W3087218857 cites W2318722737 @default.
- W3087218857 cites W2331405762 @default.
- W3087218857 cites W2461785295 @default.
- W3087218857 cites W2507406348 @default.
- W3087218857 cites W2516908105 @default.
- W3087218857 cites W2523314117 @default.
- W3087218857 cites W2528735030 @default.
- W3087218857 cites W2533728200 @default.
- W3087218857 cites W2560332898 @default.
- W3087218857 cites W2580411523 @default.
- W3087218857 cites W2594983482 @default.
- W3087218857 cites W2605748582 @default.
- W3087218857 cites W2745252600 @default.
- W3087218857 cites W2750063257 @default.
- W3087218857 cites W2755639092 @default.
- W3087218857 cites W2781950944 @default.
- W3087218857 cites W2784200684 @default.
- W3087218857 cites W2790292783 @default.
- W3087218857 cites W2800724926 @default.
- W3087218857 cites W2888289032 @default.
- W3087218857 cites W2891367289 @default.
- W3087218857 cites W2895022036 @default.
- W3087218857 cites W2901289108 @default.
- W3087218857 cites W2903522925 @default.
- W3087218857 cites W2907900959 @default.
- W3087218857 cites W2908871054 @default.
- W3087218857 cites W2911397239 @default.
- W3087218857 cites W2913234630 @default.
- W3087218857 cites W2941870743 @default.
- W3087218857 cites W2943998690 @default.
- W3087218857 cites W2944503899 @default.
- W3087218857 cites W2945181267 @default.
- W3087218857 cites W2946405653 @default.
- W3087218857 cites W2950528752 @default.
- W3087218857 cites W2954137730 @default.
- W3087218857 cites W2969493985 @default.
- W3087218857 cites W2969759954 @default.
- W3087218857 cites W2971898682 @default.
- W3087218857 cites W2978297697 @default.
- W3087218857 cites W2991011071 @default.
- W3087218857 cites W2995400468 @default.
- W3087218857 cites W3000471428 @default.
- W3087218857 cites W3010148486 @default.
- W3087218857 cites W3019179869 @default.
- W3087218857 cites W3025688758 @default.
- W3087218857 cites W3102680783 @default.
- W3087218857 doi "https://doi.org/10.1016/j.memsci.2020.118735" @default.
- W3087218857 hasPublicationYear "2021" @default.
- W3087218857 type Work @default.
- W3087218857 sameAs 3087218857 @default.
- W3087218857 citedByCount "22" @default.
- W3087218857 countsByYear W30872188572020 @default.
- W3087218857 countsByYear W30872188572021 @default.
- W3087218857 countsByYear W30872188572022 @default.
- W3087218857 countsByYear W30872188572023 @default.
- W3087218857 crossrefType "journal-article" @default.
- W3087218857 hasAuthorship W3087218857A5007737530 @default.
- W3087218857 hasAuthorship W3087218857A5008884053 @default.
- W3087218857 hasAuthorship W3087218857A5027923393 @default.
- W3087218857 hasAuthorship W3087218857A5043481897 @default.
- W3087218857 hasAuthorship W3087218857A5046889467 @default.
- W3087218857 hasAuthorship W3087218857A5061541506 @default.
- W3087218857 hasConcept C121332964 @default.
- W3087218857 hasConcept C147597530 @default.