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- W3087495587 abstract "Photoelectrocatalytic oxidation provides a technically applicable way for solar-chemical synthesis, but its efficiency and selectivity are moderate. Herein, a microfluidic photoelectrochemical architecture with 3-D microflow channels is constructed by interfacial engineering of defective WO3/TiO2 heterostructures on porous carbon fibers. Kelvin probe force microscopy and photoluminescence imaging visually evidence the charge accumulation sites on the nanojunction. This efficient charge separation contributes to a 3-fold enhancement in the yield of glyceraldehyde and 1,3-dihydroxyacetone during glycerol upgrading, together with nearly doubled production of high value-added KA oil and S2O82− oxidant through cyclohexane and HSO4− oxidization, respectively. More importantly, the microfluidic platform with enhanced mass transfer exhibits a typical reaction selectivity of 85 %, which is much higher than the conventional planar protocol. Integrating this microfluidic photoanode with an oxygen reduction cathode leads to a self-sustained photocatalytic fuel cell with remarkably high open-circuit voltage (0.9 V) and short-circuit current (1.2 mA cm−2)." @default.
- W3087495587 created "2020-09-25" @default.
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- W3087495587 date "2021-03-01" @default.
- W3087495587 modified "2023-10-18" @default.
- W3087495587 title "Interface-modulated nanojunction and microfluidic platform for photoelectrocatalytic chemicals upgrading" @default.
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- W3087495587 doi "https://doi.org/10.1016/j.apcatb.2020.119541" @default.
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